A highly efficient Au-MoS2 nanocatalyst for tunable piezocatalytic and photocatalytic water disinfection

Publication date: March 2019Source: Nano Energy, Volume 57Author(s): Ting-Mao Chou, Shuen-Wen Chan, Yu-Jiung Lin, Po-Kang Yang, Chia-Chen Liu, Yu-Jhen Lin, Jyh-Ming Wu, Jyun-Ting Lee, Zong-Hong LinAbstractClean water is essential in our daily life. However, nearly one billion people are forced to drink water contaminated with bacteria, leading to diarrhea, dehydration, and even death. Previously, various photocatalysts have been applied to replace high-cost and highly toxic methods for sewage treatment. Nevertheless, the requirement of external light sources limits their application. Herein, we develop a new type of nanocatalyst based on single- and few-layered molybdenum disulfide (MoS2) nanosheets (NSs) that can catalyze the generation of reactive oxygen species (ROS) to inactivate bacteria either through a piezoelectric effect (mechanical vibration) or photocatalytic effect (light irradiation). After 60 min of mechanical vibration or visible-light irradiation, the MoS2 NSs can reduce Escherichia coli (E. Coli) by 99.999%. In addition, the ROS generation efficiency and bacterial disinfection performance of the catalyst can be enhanced by depositing Au nanoparticles (NPs) on MoS2 NSs. The period of mechanical vibration or visible-light irradiation that achieves the same 99.999% reduction in E. coli is shortened to 45 min. Moreover, a hybridization of the piezoelectric and photocatalytic effects results in a performance superior to that obtained with the individual effect...
Source: Nano Energy - Category: Nanotechnology Source Type: research