First simultaneous detection of helium and tritium inside bubbles in beryllium

Publication date: Available online 20 September 2019Source: MicronAuthor(s): M. Klimenkov, P. Vladimirov, J. Hoffmann, N. Zimber, A. Möslang, V. KuksenkoAbstractElectron energy loss spectroscopy (EELS) was applied to detect and analyze quantitatively helium (He) and tritium (3H) enclosed inside bubbles in irradiated beryllium. Both gases were formed in beryllium under neutron irradiation as a consequence of neutron-induced transmutation reactions. They were detected for the first time as pronounced peaks at 13.0 eV for 3H and 22.4 eV for He in EELS spectra collected from flat hexagonal bubbles. An adhesion of 3H or formation of thin beryllium hydride layers on the internal basal surfaces was observed. The number densities of both gases were estimated using electron scattering cross-section and intensities obtained from EELS spectra. The number density values estimated for various bubbles fluctuate from 4 to 15 at/nm3 for He and from 4 to 10 molecules/nm3 for 3H2. Lower gas number density was measured inside large bubbles. The observed higher density of tritium at inner walls of bubbles seems to confirm very recent ab initio calculations of the interaction of hydrogen isotopes with beryllium surfaces.

Source: Micron - September 21, 2019 Category: Biology Source Type: research